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<journal-meta>
<journal-id journal-id-type="publisher-id">Front. Astron. Space Sci.</journal-id>
<journal-title-group>
<journal-title>Frontiers in Astronomy and Space Sciences</journal-title>
<abbrev-journal-title abbrev-type="pubmed">Front. Astron. Space Sci.</abbrev-journal-title>
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<issn pub-type="epub">2296-987X</issn>
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<article-id pub-id-type="publisher-id">1738959</article-id>
<article-id pub-id-type="doi">10.3389/fspas.2025.1738959</article-id>
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<subj-group subj-group-type="heading">
<subject>Original Research</subject>
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<title-group>
<article-title>Long-wavelength UV-LEDs and charge management in the detection of gravitational waves in space</article-title>
<alt-title alt-title-type="left-running-head">Jia et al.</alt-title>
<alt-title alt-title-type="right-running-head">
<ext-link ext-link-type="uri" xlink:href="https://doi.org/10.3389/fspas.2025.1738959">10.3389/fspas.2025.1738959</ext-link>
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<contrib contrib-type="author">
<name>
<surname>Jia</surname>
<given-names>Yuandong</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
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<xref ref-type="aff" rid="aff2">
<sup>2</sup>
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<name>
<surname>Zhang</surname>
<given-names>Yinbowen</given-names>
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<xref ref-type="aff" rid="aff2">
<sup>2</sup>
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<name>
<surname>Wang</surname>
<given-names>Suwen</given-names>
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<xref ref-type="aff" rid="aff3">
<sup>3</sup>
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<name>
<surname>Chai</surname>
<given-names>Guozhi</given-names>
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<sup>2</sup>
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<contrib contrib-type="author">
<name>
<surname>Zhang</surname>
<given-names>Zemin</given-names>
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<sup>2</sup>
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<surname>Zhang</surname>
<given-names>Yi</given-names>
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<sup>4</sup>
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<surname>Li</surname>
<given-names>Hongxin</given-names>
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<sup>5</sup>
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<name>
<surname>Huang</surname>
<given-names>Shuanglin</given-names>
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<sup>6</sup>
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<surname>Huo</surname>
<given-names>Hongqing</given-names>
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<given-names>Yun Kau</given-names>
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<sup>8</sup>
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<aff id="aff1">
<label>1</label>
<institution>School of Physics and Photoelectric Engineering, Key Laboratory of Gravitational Wave Precision Measurement of Zhejiang Province, Taiji Laboratory for Gravitational Wave Universe, Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences</institution>, <city>Hangzhou</city>, <country country="CN">China</country>
</aff>
<aff id="aff2">
<label>2</label>
<institution>School of Physical Science and Technology, Lanzhou University</institution>, <city>Lanzhou</city>, <country country="CN">China</country>
</aff>
<aff id="aff3">
<label>3</label>
<institution>Hainan Tropical Ocean University</institution>, <city>Sanya</city>, <country country="CN">China</country>
</aff>
<aff id="aff4">
<label>4</label>
<institution>School of Nuclear Science and Technology, Lanzhou University</institution>, <city>Lanzhou</city>, <country country="CN">China</country>
</aff>
<aff id="aff5">
<label>5</label>
<institution>School of Information Science &#x26; Engineering, Lanzhou University</institution>, <city>Lanzhou</city>, <country country="CN">China</country>
</aff>
<aff id="aff6">
<label>6</label>
<institution>Beijing Institute of Mathematical Sciences and Applications</institution>, <city>Beijing</city>, <country country="CN">China</country>
</aff>
<aff id="aff7">
<label>7</label>
<institution>Key Laboratory of Space Utilization, Technology and Engineering Center for Space Utilization, Chinese Academy of Sciences</institution>, <city>Beijing</city>, <country country="CN">China</country>
</aff>
<aff id="aff8">
<label>8</label>
<institution>Innovation Academy for Microsatellites, Key Lab for Satellite Digitalization Technology, Chinese Academy of Sciences</institution>, <city>Shanghai</city>, <country country="CN">China</country>
</aff>
<author-notes>
<corresp id="c001">
<label>&#x2a;</label>Correspondence: Hongqing Huo, <email xlink:href="mailto:huohq@lzu.edu.cn">huohq@lzu.edu.cn</email>; Zongfeng Li, <email xlink:href="mailto:lzfeng@csu.ac.cn">lzfeng@csu.ac.cn</email>
</corresp>
</author-notes>
<pub-date publication-format="electronic" date-type="pub" iso-8601-date="2025-12-19">
<day>19</day>
<month>12</month>
<year>2025</year>
</pub-date>
<pub-date publication-format="electronic" date-type="collection">
<year>2025</year>
</pub-date>
<volume>12</volume>
<elocation-id>1738959</elocation-id>
<history>
<date date-type="received">
<day>04</day>
<month>11</month>
<year>2025</year>
</date>
<date date-type="rev-recd">
<day>25</day>
<month>11</month>
<year>2025</year>
</date>
<date date-type="accepted">
<day>27</day>
<month>11</month>
<year>2025</year>
</date>
</history>
<permissions>
<copyright-statement>Copyright &#xa9; 2025 Jia, Zhang, Wang, Chai, Zhang, Zhang, Li, Huang, Huo, Li and Lau.</copyright-statement>
<copyright-year>2025</copyright-year>
<copyright-holder>Jia, Zhang, Wang, Chai, Zhang, Zhang, Li, Huang, Huo, Li and Lau</copyright-holder>
<license>
<ali:license_ref start_date="2025-12-19">https://creativecommons.org/licenses/by/4.0/</ali:license_ref>
<license-p>This is an open-access article distributed under the terms of the <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">Creative Commons Attribution License (CC BY)</ext-link>. The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.</license-p>
</license>
</permissions>
<abstract>
<p>For the charge management system in gravitational wave detection missions, a continuous discharge strategy is considered by continuously illuminating a test mass (TM) with weak light in such a way to strike a balance between the charging and discharging rates and at the same time avoids the requirement for frequent activation of charge measurements. Extending earlier experimental work on a simple parallel plate model, the present study adopts a more advanced inertial sensor model that replicates the surface properties and work function of a cubical TM in a space-based sensor. This model is used to investigate a bipolar charge management system that utilizes UV-LEDs with peak wavelengths of 269 nm, 275 nm, 280 nm, and 295 nm that are longer than the standard 255 nm commonly employed for direct TM illumination. Experimental results indicate that the 275 nm UV-LED achieves optimal performance, maintaining the TM potential closer to zero and at the same time accommodates both rapid discharge and continuous discharge strategies. The present work provides useful input in the future study of system design and optimization for the charge management system.</p>
</abstract>
<kwd-group>
<kwd>UV-LED</kwd>
<kwd>charge management</kwd>
<kwd>inertial sensors</kwd>
<kwd>passive charge control</kwd>
<kwd>discharge strategy</kwd>
</kwd-group>
<funding-group>
<funding-statement>The authors declare that financial support was received for the research and/or publication of this article. The work was supported by the National Key Research and Development Program of China (Grant No. 2021YFC2202501).</funding-statement>
</funding-group>
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<custom-meta>
<meta-name>section-in-acceptance</meta-name>
<meta-value>Astronomical Instrumentation</meta-value>
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</front>
<body>
<sec sec-type="intro" id="s1">
<label>1</label>
<title>Introduction</title>
<p>In gravitational wave detection in space, spacecraft is exposed to the heliospheric environment and subjected to continuous bombardment by high energy particles (<xref ref-type="bibr" rid="B10">Jafry et al., 1996</xref>; <xref ref-type="bibr" rid="B5">Armano et al., 2023</xref>; <xref ref-type="bibr" rid="B2">Ara&#xfa;jo et al., 2005</xref>). When the energies exceed a certain threshold, particles will penetrate the spacecraft and deposit on a TM, generating spurious acceleration noise and disturbing gravitational wave detection (<xref ref-type="bibr" rid="B7">Carbone et al., 2004</xref>; <xref ref-type="bibr" rid="B21">Sumner et al., 2020</xref>). Beginning from the Gravity Probe B (GP-B) mission and later on the LISA Pathfinder (LPF), photoelectric effect is employed as a non-contact way to neutralise charges where the mercury lamp is used as the ultraviolet (UV) light sourse (<xref ref-type="bibr" rid="B6">Buchman et al., 1995</xref>; <xref ref-type="bibr" rid="B20">Sumner et al., 2009</xref>; <xref ref-type="bibr" rid="B23">Wass et al., 2006</xref>; <xref ref-type="bibr" rid="B3">Armano et al., 2017</xref>). Instead of mercury lamp, UV-LED is considered as a better alternative for a number of technical reasons in the upcoming LISA and the prospective Chinese missions, such as <xref ref-type="bibr" rid="B15">Olatunde et al. (2015)</xref>, <xref ref-type="bibr" rid="B9">Hu and Wu (2017)</xref>, and <xref ref-type="bibr" rid="B14">Luo et al. (2016)</xref>. UV-LED based charge management systems are now widely studied, and Stanford University has successfully demonstrated charge management system with UV-LEDs in space (<xref ref-type="bibr" rid="B18">Saraf et al., 2016</xref>; <xref ref-type="bibr" rid="B8">Hollington et al., 2015</xref>; <xref ref-type="bibr" rid="B25">Yang et al., 2020</xref>; <xref ref-type="bibr" rid="B22">Wang et al., 2022</xref>).</p>
<p>During a solar cycle, charge control strategies vary with particle flux intensity. Among them, continuous discharge is used to balance the charging-discharging rates, typically suited for the ascending and descending phase of a solar cycle in which particle flux is predominantly due to galactic cosmic rays and the solar activity is low. A continuous discharge method employing dual UV light sources was proposed to illuminate both the TM and the electrode housing, effectively maintaining the TM potential near zero (<xref ref-type="bibr" rid="B16">Pi et al., 2023</xref>; <xref ref-type="bibr" rid="B22">Wang et al., 2022</xref>; <xref ref-type="bibr" rid="B4">Armano et al., 2018</xref>). Previously, Wang and the Stanford group studied continuous charge management methods by employing UV light with a peak wavelength longer than the 255 nm commonly used, and they used a simplified parallel plate model derived from an inertial sensor (<xref ref-type="bibr" rid="B22">Wang et al., 2022</xref>).</p>
<p>The aim of the present work is to conduct this study by employing a more realistic model of an inertial sensor instead of a simple parallel plate model. A cubic TM is fixed within an electrode housing via insulating pillars and the surfaces are gold coated to mimic those of the LPF in terms of the work function and surface properties of the TM as well as the electrode housing. Continuous discharge requires sustained operation during solar minimum periods. However, constrained by the experimental conditions of this study, we use 4-h continuous discharge results to demonstrate in a preliminary way its performance, corresponding to the 0.1 mHz frequency band essential for space-based gravitational wave detection. A preliminary continuous charge management is then studied using multiple wavelengths of UV-LEDs. Experimental results indicate that, due to internal reflections of UV light within the electrical housing, the photoelectron emission is different from that of a parallel plate model. Further, our results show that 275 nm outperforms the standard 255 nm wavelength for both fast release of charged particles as well as for continuous charge management, it is capable of achieving smaller equilibrium potential with long time stability.</p>
<p>In the present work, we investigate the UV-LED light sources for charge management. Although these light sources have been extensively studied by a number of research groups with focus on the 255 nm wavelength. Our contribution lies in exploring longer wavelength light sources beyond conventional 255 nm, and we argue that during periods of low solar activity, the 275 nm light source seems to be a better option. This result is similar to our previous experiments based on UV micro-LED light sources (<xref ref-type="bibr" rid="B11">Jia et al., 2025</xref>), where we used four UV micro-LEDs of different wavelengths. Light sources with wavelengths longer than the 255 nm commonly used achieved a equilibrium potential closer to 0 mV, with 274 nm reaching &#x2212;10 mV. However, in the paper (<xref ref-type="bibr" rid="B11">Jia et al., 2025</xref>), we focus more on the feasibility of applying this new light source to charge management in the detection of gravitational wave in space. We conducted a characterization analysis of the new light source and verified its potential application in the space environment.</p>
<p>The present work is structured as follows. In <xref ref-type="sec" rid="s2">Section 2</xref>, charge management model based on a UV-LED with long wavelength is introduced and analyzed. In <xref ref-type="sec" rid="s3">Section 3</xref>, based on the cubic charge management system, photoelectric effect for a UV-LED with peak wavelength of 275 nm is demonstrated. Continuous charge control using UV-LEDs with different peak wavelengths will be studied in <xref ref-type="sec" rid="s4">Section 4</xref>, which will enable us to explore a method using light sources different from the standard 255 nm. The experimental results show that UV-LEDs with longer wavelengths achieve excellent long-term stability, maintaining equilibrium potentials within approximately 50 mV over a 4-h period, and achieving a charge noise level of <inline-formula id="inf1">
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</sec>
<sec id="s2">
<label>2</label>
<title>Principle of charge management</title>
<p>In this section, we will present a charge management model for long-wavelength UV-LED illumination, on the basis of which we try to understand our experimental results and perform data analysis.</p>
<p>
<xref ref-type="fig" rid="F1">Figure 1</xref> presents a schematic representation of the charge management mechanism employing long-wavelength (i.e., wavelength longer than 255 nm) UV-LED for direct illumination. The work function of Au exposed to air is approximately 4.2 eV (<xref ref-type="bibr" rid="B19">Schulte et al., 2009</xref>; <xref ref-type="bibr" rid="B12">Jiang et al., 1998</xref>). As a result, incident light with a photon energy greater than 4.2 eV (corresponding to a wavelength of less than 295 nm) is sufficient to induce photoemission for charge management. In this configuration, UV light illuminates the TM and reflects between the TM and the electrode housing (EH). Photoelectrons are subsequently emitted from both gold-coated surfaces.</p>
<fig id="F1" position="float">
<label>FIGURE 1</label>
<caption>
<p>A schematic of photoelectron migration when the potential of the TM is positive and greater than the initial kinetic energy of the photoelectrons.</p>
</caption>
<graphic xlink:href="fspas-12-1738959-g001.tif">
<alt-text content-type="machine-generated">Diagram illustrating electron movement between two layers labeled EH and TM (VTM &#x3E; 0), with electrons represented as &#x22;e-&#x22; in circles. Arrows indicate paths and interactions with a UV-LED emitting light from the right side.</alt-text>
</graphic>
</fig>
<p>Consider the case in which the potential of the TM is positive and greater than the initial kinetic energy of the photoelectrons, where the electrode housing (including its mounted electrodes) is grounded. The presence of the local electric field causes photoelectrons to migrate to the TM, thereby reducing its potential, as shown in <xref ref-type="fig" rid="F1">Figure 1</xref>. When the potential approaches zero and becomes comparable to the initial kinetic energy of the photoelectrons, the photoelectron flow between the TM and the electrode housing reaches an equilibrium state. At this point, the TM attains a stable potential, as illustrated in <xref ref-type="fig" rid="F2">Figure 2</xref>. A similar process occurs when the initial TM charge is negative. As the wavelength of the incident light increases, the photon energy decreases, which correspondingly reduces the kinetic energy of the generated photoelectrons. Thereby, a smaller equilibrium potential of the TM can be achieved.</p>
<fig id="F2" position="float">
<label>FIGURE 2</label>
<caption>
<p>A schematic of photoelectron migration when the potential of the TM approaches zero and becomes comparable to the initial kinetic energy of the photoelectrons.</p>
</caption>
<graphic xlink:href="fspas-12-1738959-g002.tif">
<alt-text content-type="machine-generated">Diagram depicting the mechanism of electron interaction in a membrane structure. Electrons, indicated by circles with &#x22;e-&#x22;, are shown moving across EH and TM regions, represented by yellow bars. Dotted and solid arrows illustrate electron paths, reflecting off boundaries and interacting with a UV-LED source emitting purple light.</alt-text>
</graphic>
</fig>
<p>The application of a bias voltage (<inline-formula id="inf2">
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<mml:mrow>
<mml:mi>&#x3c4;</mml:mi>
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</mml:mrow>
</mml:msup>
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<mml:msub>
<mml:mrow>
<mml:mi>V</mml:mi>
</mml:mrow>
<mml:mrow>
<mml:mtext>eq</mml:mtext>
</mml:mrow>
</mml:msub>
<mml:mrow>
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<label>(1)</label>
</disp-formula>where <inline-formula id="inf3">
<mml:math id="m4">
<mml:mrow>
<mml:mi>&#x3c4;</mml:mi>
</mml:mrow>
</mml:math>
</inline-formula> is the time constant that reflects the potential variation rate of the TM, and <inline-formula id="inf4">
<mml:math id="m5">
<mml:mrow>
<mml:msub>
<mml:mrow>
<mml:mi mathvariant="normal">V</mml:mi>
</mml:mrow>
<mml:mrow>
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<mml:mi mathvariant="normal">q</mml:mi>
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</mml:mrow>
</mml:mrow>
</mml:math>
</inline-formula> is the equilibrium potential to which the TM will settle under a given bias voltage after prolonged illumination.</p>
</sec>
<sec id="s3">
<label>3</label>
<title>Ground experiments of charge management</title>
<sec id="s3-1">
<label>3.1</label>
<title>Experimental setup</title>
<p>In this work, instead of the parallel plate model, we conducted experiments using a cubic TM enclosed in an electrical housing, as in the case of the LISA Pathfinder mission. This enables us to evaluate the performance of UV-LEDs in a setting that closely resembles that on orbit.</p>
<p>
<xref ref-type="fig" rid="F3">Figure 3</xref> illustrates the experiment setup for validating long-wavelength UV-LED based charge management systems. The vacuum chamber maintained an operational pressure on the order of <inline-formula id="inf5">
<mml:math id="m6">
<mml:mrow>
<mml:mn>1</mml:mn>
<mml:msup>
<mml:mrow>
<mml:mn>0</mml:mn>
</mml:mrow>
<mml:mrow>
<mml:mo>&#x2212;</mml:mo>
<mml:mn>4</mml:mn>
</mml:mrow>
</mml:msup>
</mml:mrow>
</mml:math>
</inline-formula> Pa throughout testing. The electrical housing model was designed to mimic the inertial sensor of LISA Pathfinder, featuring a measured TM-to-surroundings capacitance of 28.8 pF. Both the surface of the TM and the inner surface of the electrode housing were gold-coated to a thickness of 500 nm (<xref ref-type="bibr" rid="B17">Saraf et al., 2014</xref>). The TM was fixed inside the electrode housing using insulated Ultem-1000 holding tubes, which provided a TM-to-EH resistance on the order of <inline-formula id="inf6">
<mml:math id="m7">
<mml:mrow>
<mml:mn>1</mml:mn>
<mml:msup>
<mml:mrow>
<mml:mn>0</mml:mn>
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<mml:mrow>
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<mml:mspace width="0.3333em"/>
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</mml:mrow>
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</inline-formula>. UV-LEDs were mounted at the upper vertices of the housing, providing direct illumination on the TM. A contact probe mounted at the centre of the upper surface of the TM was used for real-time potential measurements with an accuracy of 0.1 mV, while the bias electrode was either grounded or connected to an external voltage source to provide a bias potential. This configuration deviates from the previous simple two parallel plates model and allows for a comprehensive analysis of the charge management process under conditions that closely mimic those encountered in actual space missions.</p>
<fig id="F3" position="float">
<label>FIGURE 3</label>
<caption>
<p>Experiment setup of the charge management system. <bold>(a)</bold> Schematic. <bold>(b)</bold> Photograph.</p>
</caption>
<graphic xlink:href="fspas-12-1738959-g003.tif">
<alt-text content-type="machine-generated">Diagram and photograph of an electrode setup. In the diagram (a), components include a test mass (TM), probe, UV-LED, electrode housing, and bias electrodes. The photograph (b) depicts the actual device with labeled features including the probe, UV-LED holes, electrode housing, test mass, and bias electrodes.</alt-text>
</graphic>
</fig>
<p>
<xref ref-type="fig" rid="F4">Figure 4</xref> presents the emission spectra and optical power versus current (P-I) of the five UV-LEDs used in this study. During the P-I curve measurements, the power meter was positioned at a distance of 3 cm from the UV-LEDs. <xref ref-type="table" rid="T1">Table 1</xref> summarizes the peak wavelengths and full width at half maximum (FWHM) values for all five UV-LEDs.</p>
<fig id="F4" position="float">
<label>FIGURE 4</label>
<caption>
<p>Characteristic performance of the five UV-LEDs in the experiment. <bold>(a)</bold> Emission spectra. <bold>(b)</bold> P-I curve.</p>
</caption>
<graphic xlink:href="fspas-12-1738959-g004.tif">
<alt-text content-type="machine-generated">Two graphs comparing LED characteristics. Graph (a) shows normalized intensity versus wavelength for LEDs with peaks at 255, 265, 275, 285, and 295 nm, each with distinct curves. Graph (b) depicts optical power against current, with LED_295 showing the highest power increase, while LED_255 maintains the lowest.</alt-text>
</graphic>
</fig>
<table-wrap id="T1" position="float">
<label>TABLE 1</label>
<caption>
<p>Characteristics of the UV-LEDs used in the experiment.</p>
</caption>
<table>
<thead valign="top">
<tr>
<th align="center">LED</th>
<th align="center">Peak wavelength (nm)</th>
<th align="center">FWHM(nm)</th>
<th align="center">Manufacturer</th>
<th align="center">Part number</th>
</tr>
</thead>
<tbody valign="top">
<tr>
<td align="center">LED_255</td>
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<td align="center">
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<td align="center">NewOpto</td>
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<inline-formula id="inf9">
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<td align="center">
<inline-formula id="inf10">
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</inline-formula>
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<td align="center">NewOpto</td>
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<td align="center">
<inline-formula id="inf11">
<mml:math id="m12">
<mml:mrow>
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<mml:mo>&#xb1;</mml:mo>
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<td align="center">
<inline-formula id="inf12">
<mml:math id="m13">
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</inline-formula>
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<td align="center">NewOpto</td>
<td align="center">UVLED275-TO39HS</td>
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<tr>
<td align="center">LED_285</td>
<td align="center">
<inline-formula id="inf13">
<mml:math id="m14">
<mml:mrow>
<mml:mn>280.3</mml:mn>
<mml:mo>&#xb1;</mml:mo>
<mml:mn>0.5</mml:mn>
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</inline-formula>
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<td align="center">
<inline-formula id="inf14">
<mml:math id="m15">
<mml:mrow>
<mml:mn>13</mml:mn>
<mml:mo>&#xb1;</mml:mo>
<mml:mn>1</mml:mn>
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</mml:math>
</inline-formula>
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<td align="center">NewOpto</td>
<td align="center">UVLED285-TO39HS</td>
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<tr>
<td align="center">LED_295</td>
<td align="center">
<inline-formula id="inf15">
<mml:math id="m16">
<mml:mrow>
<mml:mn>296.3</mml:mn>
<mml:mo>&#xb1;</mml:mo>
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<td align="center">
<inline-formula id="inf16">
<mml:math id="m17">
<mml:mrow>
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</inline-formula>
</td>
<td align="center">NewOpto</td>
<td align="center">UVLED295-TO39HS</td>
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</tbody>
</table>
</table-wrap>
</sec>
<sec id="s3-2">
<label>3.2</label>
<title>Photoelectrons emission</title>
<p>To study the charge control capability of the system, two experimental runs were conducted using the LED_275. In these experiments, an increase in the potential of the TM was defined as charging, while a decrease was defined as discharging. <xref ref-type="fig" rid="F5">Figure 5</xref> illustrates the correlation between the bias electrode potential (<inline-formula id="inf17">
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</inline-formula>) and the TM potential (<inline-formula id="inf18">
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<mml:mi>V</mml:mi>
</mml:mrow>
<mml:mrow>
<mml:mtext>TM</mml:mtext>
</mml:mrow>
</mml:msub>
</mml:mrow>
</mml:math>
</inline-formula>), while the UV-LED drive current was maintained at 10 mA during the measurements.</p>
<fig id="F5" position="float">
<label>FIGURE 5</label>
<caption>
<p>Demonstration of the variation of <inline-formula id="inf19">
<mml:math id="m20">
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</inline-formula> affected by <inline-formula id="inf20">
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</inline-formula> under the illumination of LED_275. <bold>(a)</bold> <inline-formula id="inf21">
<mml:math id="m22">
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<mml:msub>
<mml:mrow>
<mml:mi>V</mml:mi>
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</mml:mrow>
</mml:math>
</inline-formula> as a function of time with <inline-formula id="inf22">
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</inline-formula> varied from &#x2212;2 V to 2 V in steps of 0.5 V. <bold>(b)</bold> <inline-formula id="inf23">
<mml:math id="m24">
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</inline-formula> as a function of <inline-formula id="inf24">
<mml:math id="m25">
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</mml:mrow>
</mml:math>
</inline-formula>.</p>
</caption>
<graphic xlink:href="fspas-12-1738959-g005.tif">
<alt-text content-type="machine-generated">Panel a shows a graph of TM potential in volts against time in seconds, displaying a stepped, symmetric pattern peaking at two volts. Panel b displays a linear graph of V_eq in volts versus V_Bias in volts, showing a direct proportionality with a positive slope.</alt-text>
</graphic>
</fig>
<p>A continuous test was conducted by sweeping <inline-formula id="inf25">
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</inline-formula> from 0 V to &#x2b;2 V, then to &#x2212;2 V, and finally returning to 0 V in steps of 0.5 V. Each voltage setting was maintained for 300 s while monitoring <inline-formula id="inf26">
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</mml:mrow>
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</inline-formula> until reaching equilibrium (<xref ref-type="fig" rid="F5">Figure 5a</xref>). Based on (1), the equilibrium potentials of the TM <inline-formula id="inf27">
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</inline-formula> configurations are plotted in <xref ref-type="fig" rid="F5">Figure 5b</xref>, where the solid line represents the fit to the data as shown in <xref ref-type="disp-formula" rid="e2">Equation 2</xref>:<disp-formula id="e2">
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<label>(2)</label>
</disp-formula>
</p>
<p>The <inline-formula id="inf29">
<mml:math id="m31">
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<mml:msup>
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<mml:mi>R</mml:mi>
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<mml:mrow>
<mml:mn>2</mml:mn>
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</inline-formula> of the fitting is 0.99989, the slope is 0.948 with a 95% confidence interval (CI) of [0.939, 0.957], and the intercept is 0.005 V with a 95% CI of [&#x2212;0.006, 0.017] V. The charge management system performance was also influenced by the UV-LED drive current. In this experiment, the LED_275 drive current was set to 10 mA, 15 mA and 20 mA respectively while the bias electrode was either grounded or set to <inline-formula id="inf30">
<mml:math id="m32">
<mml:mrow>
<mml:msub>
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<mml:mi>V</mml:mi>
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</mml:msub>
<mml:mo>&#x3d;</mml:mo>
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</inline-formula> 1 V. The corresponding TM potential variations are presented in <xref ref-type="fig" rid="F6">Figure 6</xref>. The experimental results reveal an inverse relationship between the UV-LED drive current and the stabilization time of the TM potential, while the equilibrium potential is independent of it. <xref ref-type="table" rid="T2">Table 2</xref> summarizes the maxima variation of TM potential at the start of discharge <inline-formula id="inf31">
<mml:math id="m33">
<mml:mrow>
<mml:msup>
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<mml:mo>&#x2212;</mml:mo>
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</inline-formula> and charging <inline-formula id="inf32">
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<mml:mrow>
<mml:msup>
<mml:mrow>
<mml:mrow>
<mml:mo stretchy="false">(</mml:mo>
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</inline-formula> with about 5% uncertainty for the three sets of drive current. It should be noted that the discharge rate differs from the charging rate by a factor of about 30. This discrepancy arises from two main aspects: first, the net photoelectron flux between the TM and the electrode housing depends on the potential polarity of the TM; second, it is influenced by the difference between the initial potential and the equilibrium potential of the TM.</p>
<fig id="F6" position="float">
<label>FIGURE 6</label>
<caption>
<p>TM potential variation for LED_275 with drive currents of 10 mA, 15 mA, and 20 mA. <bold>(a)</bold> The bias electrode was grounded. <bold>(b)</bold> The potential of bias electrode was set to 1 V.</p>
</caption>
<graphic xlink:href="fspas-12-1738959-g006.tif">
<alt-text content-type="machine-generated">Two graphs labeled 'a' and 'b' show TM Potential (V) over Time (s) for currents of 20mA, 15mA, and 10mA. Graph 'a' shows a decreasing curve, while graph 'b' shows an increasing curve. Different colors represent different current levels: blue for 20mA, red for 15mA, and yellow for 10mA.</alt-text>
</graphic>
</fig>
<table-wrap id="T2" position="float">
<label>TABLE 2</label>
<caption>
<p>Maxima of potential variations under different currents for the charging and discharging from <xref ref-type="fig" rid="F6">Figure 6</xref>.</p>
</caption>
<table>
<thead valign="top">
<tr>
<th align="center">I (mA)</th>
<th align="center">
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</mml:msup>
<mml:mrow>
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<mml:mrow>
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<inline-formula id="inf36">
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<mml:mrow>
<mml:mi>I</mml:mi>
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<td align="center">10</td>
<td align="center">84.5</td>
<td align="center">2.43</td>
<td align="center">2,314</td>
<td align="center">66.6</td>
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<tr>
<td align="center">15</td>
<td align="center">61.6</td>
<td align="center">1.78</td>
<td align="center">1793</td>
<td align="center">51.6</td>
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<tr>
<td align="center">20</td>
<td align="center">39.5</td>
<td align="center">1.13</td>
<td align="center">1,290</td>
<td align="center">37.2</td>
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</sec>
</sec>
<sec id="s4">
<label>4</label>
<title>Continuous charge control</title>
<p>In this experiment, long-wavelength UV-LEDs were used to evaluate the charge management performance. The performance was quantified by three metrics: the equilibrium potential of the TM, the stability of this potential, and the discharge rate.</p>
<p>
<xref ref-type="fig" rid="F7">Figure 7</xref> illustrates the equilibrium potential <inline-formula id="inf37">
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</inline-formula> &#x3d; 0 V) represents the primary focus of this study, with its detailed characteristics highlighted in the enlarged inset in the upper-left corner.</p>
<fig id="F7" position="float">
<label>FIGURE 7</label>
<caption>
<p>TM equilibrium potential as a function of the bias potential for different wavelength UV-LEDs.</p>
</caption>
<graphic xlink:href="fspas-12-1738959-g007.tif">
<alt-text content-type="machine-generated">Scatter plot showing \( V_{\text{eq}} \) versus \( V_{\text{Bias}} \) for different LEDs marked by colors and symbols: LED_255 (blue circle), LED_265 (orange cross), LED_275 (purple star), LED_285 (red plus), LED_295 (green square). An inset in the upper left magnifies the range from \(-0.1\) to \(0.1\) on both axes.</alt-text>
</graphic>
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<p>The equilibrium potential of the TM under zero-bias conditions (<inline-formula id="inf40">
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</inline-formula> &#x3d; 0 V) was used to quantify the charge management performance. <xref ref-type="table" rid="T3">Table 3</xref> summarizes these measurements (corresponding to the shaded insert in <xref ref-type="fig" rid="F7">Figure 7</xref>), demonstrating that direct TM illumination enables continuous charge control. The results show that all five UV-LEDs maintain the TM charge within <inline-formula id="inf41">
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</inline-formula> elementary charges (<xref ref-type="bibr" rid="B1">Antonucci et al., 2012</xref>). It should be noted that LED_255 and LED_265 achieve comparable equilibrium potentials around 50 mV, while the longer LED_275, LED_285, and LED_295) are moving the TM significantly closer to zero potential, indicating superior performance in precision charge management. It should be noted that the polarity of the equilibrium potential varies under different UV-LEDs. This is because the equilibrium potential is governed by the net photoelectron flux between the TM and the electrode housing, which in turn is influenced by factors such as the incident light wavelength, the geometry of the electrode housing, and the physical properties of the gold-coated surfaces. Therefore, further investigation through simulation is required to fully understand the behaviour of the equilibrium potential.</p>
<table-wrap id="T3" position="float">
<label>TABLE 3</label>
<caption>
<p>TM equilibrium potential under illumination by UV-LEDs of different wavelengths.</p>
</caption>
<table>
<thead valign="top">
<tr>
<th align="center">LED</th>
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<tbody valign="top">
<tr>
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<td align="center">
<inline-formula id="inf46">
<mml:math id="m48">
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<td align="center">LED_295</td>
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<p>To evaluate the temporal stability of the long-wavelength UV-LED-based charge management system, 4-h continuous tests were conducted using LED_265, LED_275, LED_285 and LED_295. During these tests, the drive current was set to 10 mA, and the bias electrode was grounded. <xref ref-type="fig" rid="F8">Figure 8a</xref> illustrates <inline-formula id="inf48">
<mml:math id="m50">
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</mml:mrow>
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<fig id="F8" position="float">
<label>FIGURE 8</label>
<caption>
<p>Experiment results of long-wavelength UV-LED-based charge management system. <bold>(a)</bold> TM potential drift about 4 h. <bold>(b)</bold> TM charge noise under the control of the LED_275.</p>
</caption>
<graphic xlink:href="fspas-12-1738959-g008.tif">
<alt-text content-type="machine-generated">Graph (a) displays flat lines representing IM potential (mV) over time for four different LEDs: 265, 275, 285, and 295, from -75 to 20 mV. Graph (b) shows a power spectral density plot with a line fluctuating between one point three and one point four cL per Hertz to the power of minus one half, over frequency ranging from 10 to the power of minus four to 10 to the power of minus two Hertz.</alt-text>
</graphic>
</fig>
<fig id="F9" position="float">
<label>FIGURE 9</label>
<caption>
<p>TM potential variations due to photoelectrons emitted by UV-LEDs with different wavelengths. <bold>(a)</bold> LED_265. <bold>(b)</bold> LED_275. <bold>(c)</bold> LED_285. <bold>(d)</bold> LED_295.</p>
</caption>
<graphic xlink:href="fspas-12-1738959-g009.tif">
<alt-text content-type="machine-generated">Graphs a to d display TM Potential in millivolts versus Time in seconds for different LED wavelengths. Each graph shows data points (blue) labeled LED_265, LED_275, LED_285, and LED_295 with corresponding trend lines (red) labeled fitting. The potential decreases rapidly and stabilizes around zero over varying time scales.</alt-text>
</graphic>
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<p>The experimental results demonstrate stable maintenance of the TM potential within <inline-formula id="inf49">
<mml:math id="m51">
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</inline-formula>100 mV of the target value over the 4-h duration, with all four wavelengths exhibiting peak-to-peak fluctuations below 2 mV. This confirms the viability of long-wavelength UV-LEDs for passive charge management in gravitational reference sensor applications. Under the control of the LED_275, the system achieved a charge noise level of <inline-formula id="inf50">
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</inline-formula> as derived from the literature (<xref ref-type="bibr" rid="B21">Sumner et al., 2020</xref>). Subsequently, we will conduct longer-duration continuous discharge experiments, including tests at lower frequency bands with both charge management on and charge management off, thereby validating its capability for sustained operation throughout the entire mission duration. And the 4-h test duration is relatively brief compared to a full space mission cycle, and additional risks may exist in long-term missions such as space gravitational wave detection (e.g., device aging, performance drift, etc.). Future ground-based experiments will be conducted over extended periods to simulate the complete mission cycle.</p>
<p>To evaluate the charging rate of <inline-formula id="inf52">
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<mml:mrow>
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<fig id="F10" position="float">
<label>FIGURE 10</label>
<caption>
<p>Experiments utilized AC excitation currents for UV-LED operation. <bold>(a)</bold> Three charge control cycles. <bold>(b)</bold> Details of the first cycle.</p>
</caption>
<graphic xlink:href="fspas-12-1738959-g010.tif">
<alt-text content-type="machine-generated">Graphs labeled &#x22;a&#x22; and &#x22;b&#x22; showing TM potential over time. Graph &#x22;a&#x22; illustrates multiple cycles of TM potential decreasing from 300 mV to -300 mV, whereas graph &#x22;b&#x22; shows a single cycle with a similar TM potential change from 300 mV to -300 mV. Time is in seconds on the x-axis, and TM potential in millivolts on the y-axis.</alt-text>
</graphic>
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<table-wrap id="T4" position="float">
<label>TABLE 4</label>
<caption>
<p>Time constant for different wavelength UV-LEDs.</p>
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<thead valign="top">
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<td align="center">
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<td align="center">
<inline-formula id="inf60">
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</td>
<td align="center">
<inline-formula id="inf62">
<mml:math id="m64">
<mml:mrow>
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<p>As shown in <xref ref-type="table" rid="T4">Table 4</xref>, the time constant after calibration increases with wavelength. The time constants of LED_285 and LED_295 are significantly larger than those of LED_265 and LED_275. Under conditions normalized to 1 mW output power and identical TM potentials, LED_265 and LED_275 stabilize the potential near equilibrium within 6 s. In contrast, LED_285 and LED_295 require approximately 30 s and over 600 s respectively, 5 times and 100 times longer than LED_265 and LED_275. This highlights a significant wavelength-dependent efficiency disparity in charge control.</p>
<p>While the preceding experiments utilized DC excitation currents for UV-LED operation, the methodology remains equally applicable in PWM mode. This is critical for space-based gravitational wave detectors, where DC charge control could introduce low-frequency noise into the mHz science band (<xref ref-type="bibr" rid="B24">Weber et al., 2007</xref>). <xref ref-type="fig" rid="F10">Figure 10a</xref> illustrates the potential variation of the TM through three consecutive charge-discharge cycles, employing LED_275 in PWM mode. The LED was driven at a current of 20 mA and modulated at 1 kHz with 50% duty cycle. The TM was alternately biased with a positive or negative initial potential, followed by UV-LED illumination until equilibrium was achieved in each case. This alternating sequence was repeated for three cycles, and the shaded area indicates periods of UV-LED activation.</p>
<p>The experimental results demonstrate consistent convergence of the TM potential to equilibrium under UV-LED activation across all three cycles, regardless of initial potential polarity. <xref ref-type="fig" rid="F10">Figure 10b</xref> details the transient behavior of the first cycle (0&#x2013;400 s), revealing charge and discharge phases from the initial potentials to equilibrium. This bipolar charge control demonstrates the robustness of the methodology, as demonstrated in the previous research (<xref ref-type="bibr" rid="B22">Wang et al., 2022</xref>; <xref ref-type="bibr" rid="B17">Saraf et al., 2014</xref>).</p>
<p>The experimental results demonstrate that for gold-coated surfaces, the LED_265 showed performance comparable to the LED_255, and the LED_275, LED_285 and LED_295 exhibit a lower equilibrium potential (within 20 mV) compared to the LED_255, while wavelengths approaching 300 nm and beyond are ineffective due to insufficient photon energy. Moreover, LED_275 seems to be an optimal candidate for the source of charge management system, not only achieving a smaller equilibrium potential compared to LED_255 and LED_265 but also demonstrating a shorter time constant than long-wavelength UV-LEDs, such as LED_285 or LED_295. It should be clarified that our approach does not entirely replace the 255 nm UV-LED with the 275 nm variant. Instead, it offers more options for neutralizing cosmic ray charging, pending on the solar activity. On board, both the 255 nm and 275 nm should be placed at the four bottom corners of the caging. Depending on the intensity of the solar energetic particles and possibly contamination of the test mass, UV-LED of appropriate wavelengths will be activated for charge management.</p>
</sec>
<sec sec-type="conclusions" id="s5">
<label>5</label>
<title>Conclusions</title>
<p>Based on a model of inertial sensor that mimics the surface properties and work function of a TM for LISA, UV-LEDs with multiple wavelengths were tested to evaluate their performance in continuous charge management, in terms of both the equilibrium potential and long-term stability. Additionally, the discharge rates (time constant) of UV-LEDs with different wavelengths were measured. The results show that LED_275 appears to be the best choice if optimizing for both these parameters. These results demonstrate that the 275 nm UV-LED is a promising candidate for the continuous charge management and at the same time for regular rapid discharge operation.</p>
<p>It is our hope that our work will provide useful input when it comes to the system design and optimisation of the charge management system in the engineering phase of a mission to detect gravitational waves in space.</p>
</sec>
</body>
<back>
<sec sec-type="data-availability" id="s6">
<title>Data availability statement</title>
<p>The original contributions presented in the study are included in the article/Supplementary Material, further inquiries can be directed to the corresponding authors.</p>
</sec>
<sec sec-type="author-contributions" id="s7">
<title>Author contributions</title>
<p>YJ: Writing &#x2013; original draft. YnZ: Writing &#x2013; original draft. SW: Writing &#x2013; review and editing, Methodology. GC: Supervision, Writing &#x2013; review and editing. ZZ: Formal Analysis, Writing &#x2013; review and editing. YiZ: Writing &#x2013; review and editing, Formal Analysis. HL: Writing &#x2013; review and editing, Formal Analysis. SH: Writing &#x2013; review and editing, Formal Analysis. HH: Writing &#x2013; review and editing, Resources, Funding acquisition. ZL: Writing &#x2013; review and editing, Resources. YL: Writing &#x2013; review and editing.</p>
</sec>
<sec sec-type="COI-statement" id="s9">
<title>Conflict of interest</title>
<p>The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.</p>
</sec>
<sec sec-type="ai-statement" id="s10">
<title>Generative AI statement</title>
<p>The authors declare that no Generative AI was used in the creation of this manuscript.</p>
<p>Any alternative text (alt text) provided alongside figures in this article has been generated by Frontiers with the support of artificial intelligence and reasonable efforts have been made to ensure accuracy, including review by the authors wherever possible. If you identify any issues, please contact us.</p>
</sec>
<sec sec-type="disclaimer" id="s11">
<title>Publisher&#x2019;s note</title>
<p>All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations, or those of the publisher, the editors and the reviewers. Any product that may be evaluated in this article, or claim that may be made by its manufacturer, is not guaranteed or endorsed by the publisher.</p>
</sec>
<fn-group>
<fn fn-type="custom" custom-type="edited-by">
<p>
<bold>Edited by:</bold> <ext-link ext-link-type="uri" xlink:href="https://loop.frontiersin.org/people/3039354/overview">Gang Wang</ext-link>, Ningbo University, China</p>
</fn>
<fn fn-type="custom" custom-type="reviewed-by">
<p>
<bold>Reviewed by:</bold> <ext-link ext-link-type="uri" xlink:href="https://loop.frontiersin.org/people/1156314/overview">Wenjie Zhao</ext-link>, National Space Science Center, Chinese Academy of Sciences (CAS), China</p>
<p>
<ext-link ext-link-type="uri" xlink:href="https://loop.frontiersin.org/people/3276714/overview">Pengfei Tian</ext-link>, Fudan University, China</p>
</fn>
</fn-group>
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